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Organic Reaction Mechanisms Overview

Chapter 3 covers the fundamentals of acids and bases, including their definitions, strengths, and roles in organic reactions. It explains various types of organic reactions, mechanisms, and the importance of electron movement in these processes. Additionally, it discusses factors affecting acidity, such as electronegativity, hybridization, and solvent effects.

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0% found this document useful (0 votes)
5 views40 pages

Organic Reaction Mechanisms Overview

Chapter 3 covers the fundamentals of acids and bases, including their definitions, strengths, and roles in organic reactions. It explains various types of organic reactions, mechanisms, and the importance of electron movement in these processes. Additionally, it discusses factors affecting acidity, such as electronegativity, hybridization, and solvent effects.

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Chapter 3

Acids & Bases


Intro to Organic Reactions & Their Mechanisms
Mechanism
• A reaction mechanism is a detailed description
of the bonding changes as a reaction proceeds
• A plausible mechanism must be consistent
with the principles of organic chemistry

2
Types of Reactions
• Addition reactions – usually found in compounds with
multiple bonds
– The  component of the multiple bond is lost as the new bonds are
formed

• Elimination reactions – atoms are lost resulting in a multiple


bond

3
Types of Reactions
• Substitution reactions – replaces one atom or part of a
molecule with another

• Rearrangements – same number of atoms present in reactant


& product; the bonds have a different arrangement

4
Mechanisms
• A mechanism describes what takes place at each
stage of a chemical reaction
• It shows how electrons move as well as how bonds
break and form
• There are two types of bond breaking
– Homolytic (symmetrical) – forms radicals

– Heterolytic (unsymmetrical) – forms ions

5
Mechanisms
• Half curved arrow ( ) shows the movement of one
electron
• Whole curved arrow ( ) shows the movement of two
electrons
• There are two types of bond forming
– Homolytic (symmetrical) – one electron from two different atoms pair
up to form a bond

– Heterolytic (unsymmetrical) – two electrons from one atom form a


bond with a second atom

6
Mechanisms
• Heterolytic bond breaking and forming are the
most common; usually happens with polar
covalent bonds
– They are sometimes called polar reactions
because they usually have one species more
negative than the other
• Terminology
– Electrophile – more positive, electron poor species
– Nucleophile – more negative, electron rich species

7
Mechanisms
• When drawing curved arrows, the nucleophile
(negative) always points toward the electrophile
(positive)
• Nucleophiles can be neutral or negatively charged
– Examples

– Almost anything that has a lone pair can be a


nucleophile

8
Mechanisms
• Electrophiles can be neutral or positively
charged
– Examples

• Some compounds can act as either a


nucleophile or an electrophile depending on
what it is reacting with

9
Acids and Bases
• Bronsted-Lowry acid – substance that donates a
proton (H+)
• Bronsted-Lowry base – substance that accepts a
proton (H+)
• Example
– HCl is a B-L acid; H2O is a B-L base

10
Acids and Bases
• Acid strength is a measure of the % ionization
• Strong acids completely dissociate (ionize) in
water
– Ex: HCl, HI, HBr, H2SO4, HNO3
• Weak acids partially dissociate (ionize) in
water; doesn’t give up a proton easily
– Ex: CH3COOH, HCN, H3PO4

11
Acids and Bases in Water
• H3O+ (hydronium) – strongest acid in water
• OH– (hydroxide) – strongest base in water
• When a strong acid or base is added to water
the form hydronium or hydroxide
• Example

12
Acids and Bases in Water
• When ionic compounds dissolve in water the
ions are solvated

• Mix HCl(aq) & NaOH(aq)

13
Lewis Acids and Bases
• Not all compounds contain hydrogen so the B-L definition
doesn’t always apply
• Lewis acid – substance that can accept a pair of electrons
• Lewis base – substance that can donate a pair of electrons

• Curved arrow indicates e- movement

14
Organic Reactions
• The attraction of oppositely charged species is
fundamental to reactivity

• The negative area of one species is attracted


to the positive area of another species

15
Carbocations & Carboanions
• Heterolysis of a carbon bond can produce
either a carbocation or carbanion

16
Carbocations & Carboanions
• Carbocations are Lewis acids and are
electrophiles (electron seeking)
• All Lewis acids are electrophiles

• Carboanions are Lewis bases & are


nucleophiles
17
How to use Curved Arrows
• Curved arrows denote electron flow from a
site of higher electron density to a site with
lower electron density
• Arrows are in the direction from the
nucleophile to the electrophile
• Example

18
Acids and Bases
• Organic acids are weak acids
• Many biological reactions involve organic
acids and bases
• Major types:
– Compounds that have H attached to an
electronegative atom
– Compounds that have H attached to a carbon next
to a C=O

19
Acids and Bases
• The strength of an acid can be expressed by the
acidity constant (Ka)

𝐴− [𝐻3 𝑂+ ]
𝐾𝑎 =
[𝐻𝐴]
• Strong acids have larger Ka values; weaker acids
have smaller Ka values
• Ka values range from 1015 to 10-60

20
Acids and Bases
• Its easier to express acidity in terms of pKa
pKa = -log(Ka)
• Strong acids: small pKa (large Ka)
• Weak acids: large pKa (small Ka)

Check out
Table 3.1 in
the book on
page 115

21
Acids & Bases
• Predicting base strength
– The stronger the acid, the weaker its conjugate
base
– The larger the pKa value of the conjugate acid, the
stronger the base

22
Acids and Bases
• Predicting acid-base reactions
– Acid-base reactions always favor the formation of
the weaker acid and weaker base
– Example 1:

– Example 2:

23
Acids and Bases
• Carboxylic acids – contain a COOH group; a
type of organic acid
– Example: acetic acid (CH3COOH)

• Organic bases – usually contain an atom that


has a lone pair of electrons (like amines)

24
Water Solubility
• Most medicines are organic compounds – they are turned into salts that
the body can absorb
• Several carboxylic acids that contain less than 5 carbons are water soluble
• Most organic compounds that have more than 5 carbons are not water
soluble

25
Bond Strength & Acidity
• The stronger the bond, the weaker the acid
• A strong acid has a weak bond – easy to lose a
proton (H+)

26
Electronegativity & Acidity
• Acidity increases as electronegativity increases
• Fluorine is the most electronegative & holds
electrons close to itself but farther away from
the other atom

• A strong acid has a weak conjugate base

27
Hybridization & Acidity
• The more S character, the more acidic

• Having more S character means that the


electrons on the anion will be lower in energy
& the anion will be more stable
28
Inductive Effects
• Electronic effects transmitted through bonds
• The effects weaken as the distance from the
group increases
• Fluorine is electron withdrawing

• C1 is more positive than C2

29
Energy Changes
• The stability of a system is inversely related to
its potential energy
• Chemical energy (energy of molecules) is a
form of potential energy
• “The more energy an object has, the less
stable it is”
• Chemists use the word stability to describe
systems – the most stable system has the
lowest energy
30
Thermodynamics Review
• ΔH = enthalpy (heat)
– Positive value = endothermic reaction
– Negative value = exothermic reaction
• ΔG = Gibbs free energy
– Positive value = reactant favored
– Negative value = product favored
• ΔS = entropy (disorder)
– Positive value = more disorder
– Negative value = more order

31
Carboxylic Acids
• If you compare a carboxylic acid to an alcohol,
why is the carboxylic acid more acidic?
• Resonance of the conjugate base – can
stabilize the negative charge by delocalizing it

32
Carboxylic Acids
• Carboxylic acids also have more inductive
effects than alcohols

• Carboxylic acids do not have as much electron


density holding onto the hydrogen

33
Substituent Effects
• Electron withdrawing groups near the
carboxylic acid can increase its acidity

• Any factor that stabilizes the conjugate base of


an acid increases the acid strength

34
Solvent Effects on Acidity
• Protic solvent – has a hydrogen attached to a strong
electronegative atom
– Example: H2O, CH3OH, NH3, etc.
• Water causes acetic acid to be more acidic when
dissolved
• Water solvates the ions & stabilizes them

35
Organic Bases
• Compounds with lone pairs have the potential
to be bases

• Proton transfer is the very first step in many


reactions

36
Organic Reaction Mechanisms

37
Acids & Bases in Non-Aqueous Solutions

• Water donates a proton to any base stronger


than hydroxide

38
Acids & Bases in Non-Aqueous Solutions

• Alcohols are good solvents because they are


less polar than water & dissolve less polar
compounds

• Bases much stronger than hydroxide:


– BuLi, EtLi, LDA (lithium diisopropylamide), NaNH2,
NaH, acetylides, & more

39
Practice Problems
• Chapter 3 (12th Ed.): 1-19, 20, 22-28, 30, 34,
35, 38, and 44

40

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