Project
Project
MOHAMMED
1 | P a g e K. AL-ZGHOOL SUPERVISED BY:
SAIF ALDEEN O. ALMASHAQBEH [Link] ABU ENNAB
Contents
Abstract ........................................................................................................................................... 1
1. Literature review...................................................................................................................... 2
1.1 Neutron reactions ............................................................................................................. 3
2. Structure of the detector .......................................................................................................... 5
2.1 Converter Part .................................................................................................................. 5
2.1.1 Boron......................................................................................................................... 5
2.1.2 Zinc ........................................................................................................................... 6
2.2 Detection Part (G-M tube)................................................................................................ 6
2.3 Shielding from gamma release (Lead) ............................................................................. 7
2.4 Protection of equipment part (Stainless Steel) ................................................................. 8
3. Neutron separation and detection ............................................................................................ 8
3.1 Introduction ...................................................................................................................... 8
3.2 The way of separating the neutrons.................................................................................. 9
3.3 Shield from gamma release by Lead .............................................................................. 11
4. MCNP5 .................................................................................................................................. 11
4.1 About the MCNP5.......................................................................................................... 11
4.2 Input code ....................................................................................................................... 12
4.3 Output .................................................................................................................................. 13
5. Results ................................................................................................................................... 22
5.1 potential scenario............................................................................................................ 22
5.1.1 Failure of the project................................................................................................... 22
5.2 Problems and potential solutions.................................................................................... 23
5.2.1 Problems ................................................................................................................. 23
5.2.2 Potential solutions ................................................................................................... 23
5.3 New potential applications ............................................................................................. 23
5.3.1 Neutron Filter .......................................................................................................... 23
5.3.2 The Depleted Fuel Conversion Unit ....................................................................... 23
References ..................................................................................................................................... 24
Abstract
This report will discuss the design and construction of a NEUTRONS SEPERATION
DETECTOR, which is designed to measure the ratio of thermal and epithermal neutrons to the
fast neutrons which can be used to measure the efficiency of the moderator in order to add a
material to the moderator and present the effect of this materials for this efficiency or we can use
it in the Fast Reactor in order to test a lot of metals and measure their efficiency and other
applications. We were supposed to build and test the project on MCNP5, but we did not have an
original version and we have a non-original version, which we cannot display the possible tracks
to display the scenario that will happen, so we will address the most prominent scenario that may
appear in this project.
According to the expected final results, we found that the project did not achieve its goal of
separating and detecting neutrons, and there were more feasible uses for it, such as the Neutron
Filter and The Depleted Fuel Conversion Unit.
It is worth noting that these two new applications are descended from the same method of work.
In the Neutron Filter, it filters neutrons with energy less than the neutrons desired energy in
experiments in which we need fast neutrinos.
And the same principle we use to convert U238 (fertile material) into Pu239 (fissile material) and
this reaction is done by fast neutrons.
Dedicated to [Link] MASADEH, who helped us in this project to use the MCNP5
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1. Literature review
Radiation is the process by which energy is emitted as either particles or waves. Broadly, it can
take the form of sound, heat, or light.
Atoms form the basic building blocks of all matter. They consist of a nucleus, made of positively-
charged protons (and sometimes neutrally-charged neutrons), and an outer cloud of electrons with
a negative charge. The positive charge of a single proton is equal to the negative charge of a single
electron.
Protons and neutrons have a relatively large size and atomic weight, whereas electrons are
extremely small and light by comparison. Due to the nature of opposite charges attracting, atoms
tend to have an equal number of protons and electrons, leaving the atom as a whole having a net
charge of zero. However, if the atom either loses or gains an electron, it becomes an ion and carries
a charge. It will seek bonds with other charged particles in order to regain a neutral balance,
potentially leading to new molecules being formed.
Ionizing radiation takes a few forms: Alpha, beta, neutron particles, gamma, and X-rays. All types
are caused by unstable atoms, which have either an excess of energy or mass (or both). In order to
reach a stable state, they must release that extra energy or mass in the form of radiation.
Ionizing radiation is not detectable by one's senses. It cannot be seen, heard, smelled, tasted, or
felt. For these reasons, simple visual inspection is insufficient to identify radioactive materials,
and radiation sources can be virtually impossible to recognize without special markings, so we use
a Radiation detector which is a device used to detect, track, or identify ionizing particles.
When talking about radiation detection instruments, there are three types of detectors that are most
commonly used depending on the specific needs of the device which are Gas-Filled Detectors,
Scintillators, and seme conductor detectors.
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1.1 Neutron reactions
Scattering
There is no energy transferred into nuclear excitation in an elastic scattering reaction between a
neutron and a target nucleus. An inelastic scattering plays an important role in slowing down
neutrons, especially at high energies and by heavy nuclei.
A neutron scattering reaction occurs when a target nucleus emits a single neutron after a neutron-
nucleus interaction. Besides, in an inelastic scattering reaction between a neutron and a target
nucleus, some energy of the incident neutron is absorbed into the recoiling nucleus and the nucleus
remains in the excited state. Thus while momentum is conserved in an inelastic collision, the
kinetic energy of the “system” is not conserved.
In inelastic neutron scattering, the incident neutron is absorbed by the target nucleus, and the
interaction takes place via compound nucleus formation. The compound nucleus emits then a
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neutron of lower kinetic energy, which leaves the original nucleus in an excited state. The nucleus
gives up excitation energy by emitting one or more gamma rays to reach its ground state.
Inelastic scattering occurs above threshold energy. This threshold energy is higher than the energy
of the first excited state of the target nucleus (due to the laws of conservation),
Absorption
The absorption reactions are reactions where the neutron is completely absorbed, and the
compound nucleus is formed. This is a very important feature because the mode of decay of such
a compound nucleus does not depend on how the compound nucleus was formed. Therefore, a
variety of emissions or decays may follow.
The absorption reactions are reactions where the neutron is completely absorbed, and the
compound nucleus is formed. This is a very important feature because the mode of decay of such
a compound nucleus does not depend on how the compound nucleus was formed. Therefore, a
variety of emissions or decays may follow.
The neutron absorption reaction is the most important type of reaction that takes place in a nuclear
reactor. The most important absorption reactions are divided into two categories:
• Radiative Capture: Most absorption reactions result in the loss of a neutron coupled with
the production of one or more gamma rays. This is denoted by 𝜎𝛾 .
• Neutron-induced Fission Reaction (σf): Some nuclei (fissionable nuclei) may undergo a
fission event, leading to two or more fission fragments (nuclei of intermediate atomic weight) and
a few neutrons. In a fissionable material, the neutron may simply be captured, or it may cause
nuclear fission. For fissionable materials, we thus divide the absorption cross-section as
𝜎𝑎 = 𝜎𝛾 + 𝜎𝑓 … … … (1)
The absorption cross-section represents the likelihood of a neutron absorption as 𝜎𝑎 . The relative
likelihoods of an absorption reaction or a neutron scattering are represented by dividing the total
cross-section into scattering and absorption cross-sections:
𝜎𝑡 = 𝜎𝑠 + 𝜎𝑎 … … … (2)
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Given a collision, 𝜎𝑎 / 𝜎𝑡 is the probability that the neutron will be absorbed, and 𝜎𝑠 / 𝜎𝑡 is the
probability that the neutron will be scattered.
Transfer
Transfer reaction is the absorption of neutrons and the production of other particles such as protons,
alpha particles, or neutrons.
2.1.1 Boron
In engineering, the most important neutron absorber is 10B, Boron is a naturally occurring chemical
element with atomic number 5 which means there are 5 protons and 5 electrons in the atomic
structure. The chemical symbol for boron is B. Significant boron concentrations occur on the Earth
in compounds known as the borate minerals. There are over 100 different borate minerals, but the
most common are borax, kernite, ulexite, etc.
11 10
Natural boron consists primarily of two stable isotopes, B (80.1%) and B (19.9%). In the
nuclear industry, boron is commonly used as a neutron absorber due to the high neutron transfer
cross-section of isotope 10B. Its (n, alpha) reaction cross-section for thermal neutrons is about 3840
barns (for 0.025 eV neutron). Isotope 11B has absorption cross-section for thermal neutrons about
10
0.005 barns (for 0.025 eV neutron). Most of (n, alpha) reactions of thermal neutrons are B (n,
alpha) 7Li reactions accompanied by 0.48 MeV gamma emission.
5|Page
The reaction products (after neutron absorption), helium and lithium, are stable isotopes.
Neutrons are not directly ionizing, and they usually have to be converted into charged particles
before they can be detected. The most common isotope for neutron converter material is 10B.
2.1.2 Zinc
Zinc is a transition earth metal with atomic number 30 which means it has 30 protons and 30
electrons in the atomic structure. The chemical symbol for boron is Zn.
70
Zinc has five natural isotopes, with mass numbers 64,66, 67, 68 and 70. Of these, Zn has an
abundance of only 0.6% and hence was omitted from the evaluation The other four isotopes were
each evaluated separately. The cross-sections so obtained were then combined together to give the
natural zinc cross-sections.
Some reasons for errors are the interaction between the zinc and neutron result neutrons, and other
errors are because of some non-desired reactions as shown in the Table below:
The different types of gas-filled detectors are ionization chambers, proportional counters, and
Geiger-Mueller (G-M) tubes. The major differentiating factor between these different types is the
6|Page
applied voltage across the detector, which determines the type of response that the detector will
register from an ionization event.
The GM-tube which we will use in our project has two main parts—a sealed tube, or chamber,
filled with gas, and an information display. Radiation enters the tube and when it collides with the
gas, it pushes an electron away from the gas atom and creates an ion pair. A wire in the middle of
the tube attracts electrons, creating other ion pairs and sending a current through the wire. The
current goes to the information display and moves a needle across a scale or makes a number
display on a screen. These devices usually provide "counts per minute," or the number of ion pairs
created every 60 seconds.
A gas-filled detector was chosen because of its low density to detect only charged particles and to
reduce the rate of detection of gamma rays resulting from the interaction between neutrons with
the materials used in this project.
Lead is a soft metal that can be easily scratched or dented. Being ductile and malleable makes lead
very easy to work with. It is a very dense metal with a density of 11.34 g/cc, approximately 4 times
the density of aluminum. Lead has a melting point of 327°C which makes it an ideal metal to cast.
There are many different alloys and purities of lead available. One of the most common is ASTM
B-29 lead, which has a minimum purity of 99.94% lead. The lead is refined to reach this level of
purity.
Lead is very effective at shielding gamma radiation. Because of the density of lead, its high atomic
number, and stable isotopes, lead is ideal for stopping gamma and x-ray radiation. For a gamma
ray from a Colbalt-60 source, pure lead has a Half-Value Layer (HVL – the thickness of shielding
required to reduce the level of radiation by 50%) of approximately 12.5 mm (0.49 in). A lead shield
will be thinner than a steel or concrete shield of the same effectiveness in shielding a Co60 source.
7|Page
2.4 Protection of equipment part (Stainless Steel)
Stainless steel is a common choice in different industries because of its strong resistance to
corrosion. Furthermore, stainless steel’s durability makes it a top choice among industry experts.
Unlike other alloys, stainless steel does not readily react to corrosive agents like air or water and
exhibit signs of corrosion such as staining.
Stainless steel’s corrosion-resistant properties are due to the chromium content, which should be
a minimum of 10.5 percent per mass. Chromium creates a passive film of chromium oxide, a
compound that blocks the chemical reaction between oxygen and the steel surface.
Stainless steel’s melting point falls between 2550 and 2790°F or 1400 and 1530°C.
The melting point of a particular type of stainless steel depends upon its exact chemical
composition. The major elements composing stainless steel are iron, chromium, and nickel.
Pure iron has a fixed melting point of 1535°C, chromium of 1890°C, and nickel of 1453°C.
Compare those numbers to the 1400-1530°C range for stainless steel.
In this report, we will look at a different use of the detector. Where detector will separate the fast
neutrons from the Thermal and Epithermal through a layer of boron interacting with Thermal
neutrons forming alpha particle and 7Li. While a layer of zinc interacts with fast neutrons, forming
a charged particle and another atom.
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3.2 The way of separating the neutrons
The design of the NEUTRONS SEPERATION DETECTOR is a four-layer cylinder, the thickness
of each layer was determined by calculating Half Value Layer (HVL), and we chose boron and
zinc based on their high cross-section. If we consider that the source of the neutrons is
Polyenergetic, the energy of the neutrons created can range from 0 to 2 Mev (Heterogeneous).
When the neutrons enter the detector, the thermal neutrons and the epithermal interact with the
first layer (boron), the nuclear reaction produces helium nuclei (α-particle), lithium-7 nuclei, and
energy.
The second and fourth layers contain air with a thickness of 10 cm, and the charged particle is
collected by applying a potential difference and creating a reading through an electrical circuit
similar to that of Geiger-Muller. Fast neutrons will be stopped by a layer of zinc which has a high
cross-section of 2.6 barns. The reaction of the fast neutron with it produces a proton and copper
64Zn (n, p) 64Cu. and the detector housing has been added. Below is a calculation of the thickness
of each layer.
From the fact of the density of boron is 2.34 g/cm3 and the molar mass is 10.012937 amu we find
the atomic density of boron:
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𝐴𝑉 ∗ 𝜌
𝑁= … … … (3)
𝑀
Where:
N: atomic density
𝐴𝑉 : Avogadro’s number
M: molar mass
ρ: density of material
Where:
Σ: macroscopic cross-section
σ: microscopic cross-section
ln(2)
𝐻𝑉𝐿 = … … … (5)
Σ
Where:
ln(2)
𝐻𝑉𝐿 = = 4.764657972𝑐𝑚
0.145476797
3HVL=14.2939739159=14.3cm
From the fact of the density of Zinc is 7.133 g/cm^3 and the molar mass is 65.39 amu we find the
atomic density of Zinc:
3HVL=12.1740665768=12.2cm
ln(2)
𝐻𝑉𝐿 = … … … (6)
Σ
∗ 𝜌
𝜌
ln(2)
𝐻𝑉𝐿 = = 0.3783781671𝑐𝑚
11.35 ∗ 0.1614
3HVL=1.1351345014=1.14cm
Not that we add stainless steel thickness of 0.5cm as a Housing to the detector
4. MCNP5
4.1 About the MCNP5
The MCNP Code, developed and maintained by Los Alamos National Laboratory, is the
internationally recognized code for analyzing the transport of neutrons and gamma rays (hence NP
for neutral particles) by the Monte Carlo method (hence MC). The code deals with transport of
neutrons, gamma rays, and coupled transport, i.e., transport of secondary gamma rays resulting
from neutron interactions. The MCNP code can also treat the transport of electrons, both primary
source electrons and secondary electrons created in gamma-ray interactions.
One of the most important blocks we use is data specifications This block of input cards defines
the type of particles, problem materials, radiation sources, how results are to be scored (or tallied),
the level of detail for the physics of particle interactions, variance reduction techniques, cross
section libraries, the amount and type of output, and much more. In short, this third input block
provides almost all problem specifications other than the geometry.
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A summary of available tallies in MCNP5 is given below in table 2:
Table 2 Types of tallies available in MCNP. the type of particle tallied is donated by pl.
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33. 28000. -0.12 42000. -0.025
34. m171 82000. -1 $Lead
35. m365 30000. -1 $Zinc
36. imp:n 1 7r $ 1, 8
37. sdef pos -24.25 0 0
38. f6:n 1 3
39. e6 0 10i 2
40. nps 1000000
41.
4.3 Output
By default, only a small portion of all the possible output is produced. Always output are (1) input
file listing, (2) summary of particle loss/creation, (3) summary of KCODE cycles (if KCODE is
used), (4) tallies (if used), and (5) tally fluctuations charts. In addition, certain output tables deemed
basic are always produced.
Other default tables are also generated unless turned off by the PRINT command. The various
MCNP tables are listed below in Table 3:
Table 3 output tables available in MCNP. (d)=default;(b) =basic.
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The following code is the output for our input showed by the MCNP5:
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29- 28000. -0.12 42000. -0.025
30- m171 82000. -1 $Lead
31- m365 30000. -1 $Zinc
32- imp:n 1 7r $ 1, 8
33- sdef pos -24.25 0 0
34- f6:n 1 3
35- e6 0 10i 2
36- nps 1000000
37- print table 30
fatal error. illegal entry: table
1source
print table 10
cel 0.0000E+00
sur 0.0000E+00
erg 1.4000E+01
tme 0.0000E+00
dir isotropic
pos -2.4250E+01 0.0000E+00 0.0000E+00
x 0.0000E+00
y 0.0000E+00
z 0.0000E+00
rad 0.0000E+00
ext 0.0000E+00
axs 0.0000E+00 0.0000E+00 0.0000E+00
vec 0.0000E+00 0.0000E+00 0.0000E+00
ccc 0.0000E+00
nrm 1.0000E+00
ara 0.0000E+00
wgt 1.0000E+00
eff 1.0000E-02
par 0.0000E+00
tr 0.0000E+00
1tally 6
print table 30
tally type 6 track length estimate of heating.
tally for neutrons
energy bins
0.00000E+00 to 0.00000E+00 mev
0.00000E+00 to 1.81818E-01 mev
1.81818E-01 to 3.63636E-01 mev
3.63636E-01 to 5.45455E-01 mev
5.45455E-01 to 7.27273E-01 mev
7.27273E-01 to 9.09091E-01 mev
9.09091E-01 to 1.09091E+00 mev
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1.09091E+00 to 1.27273E+00 mev
1.27273E+00 to 1.45455E+00 mev
1.45455E+00 to 1.63636E+00 mev
1.63636E+00 to 1.81818E+00 mev
1.81818E+00 to 2.00000E+00 mev
total bin
1material composition
print table 40
material
number component nuclide, atom fraction
material
number component nuclide, mass fraction
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5 5 8.65494E-02 8.00000E+00 0.00000E+00 4.95225E+02
3.96180E+03 1
6 6 3.29849E-02 1.13500E+01 0.00000E+00 8.55994E+02
9.71553E+03 1
7 7 0.00000E+00 0.00000E+00 0.00000E+00 6.35143E+04
0.00000E+00 1
8 8 0.00000E+00 0.00000E+00 0.00000E+00 0.00000E+00
0.00000E+00 0 infinite
1surface areas
print table 50
1 1 0.00000E+00 1.06349E+03
2 2 0.00000E+00 9.17408E+02
3 3 0.00000E+00 5.84336E+02
4 4 0.00000E+00 4.16248E+01
5 5 0.00000E+00 4.16248E+01
6 6 0.00000E+00 1.25664E+01
7 7 0.00000E+00 1.25664E+01
8 8 0.00000E+00 1.25664E+01
9 10 0.00000E+00 7.85398E+03
1cells
print table 60
atom gram
neutron
cell mat density density volume mass pieces
importance
1 1 cx 3.6400000E+00
2 2 cx 3.1400000E+00
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3 3 cx 2.0000000E+00
4 4 px -2.3250000E+01
5 5 px 2.3250000E+01
6 6 px -8.9500000E+00
7 7 px 1.0500000E+00
8 8 px 1.3250000E+01
9 10 so 2.5000000E+01
1 cell temperatures in mev for the free-gas thermal neutron treatment.
print table 72
***************************************************
* Random Number Generator = 1 *
* Random Number Seed = 19073486328125 *
* Random Number Multiplier = 19073486328125 *
* Random Number Adder = 0 *
* Random Number Bits Used = 48 *
* Random Number Stride = 152917 *
***************************************************
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93237 183.67 94238 186.65
94239 189.44 94240 186.36
94241 188.99 94242 185.98
94243 187.48 95241 190.83
95242 190.54 95243 190.25
96242 190.49 96244 190.49
other 180.00
cheap
dec
plot
mcplot
gkssim
xlib
default datapath: C:\Program Files (x86)\LANL\MCNPDATA
C:\Progra~1\LANL\MCNPdata
1cross-section tables
print table 100
table length
18000.59c 2059
(1800) 06/19/82
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tables from file rmccs
total 976853
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Figure 3 the section of the layers of the detector simulated using AutoCAD
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5. Results
We were supposed to build and test the project on MCNP5, but we did not have an original version
and we have a non-original version, which we cannot display the possible tracks to display the
scenario that will happen, so we will address the most prominent scenario that may appear in this
project.
Figure 5 Variation of range of proton as a function of kinetic energy in the zinc borophosphate glasses [5]
note that alpha particle travel distances in different materials are calculated by finding the mean
range of travel distance in which the intensity of alpha particles drops by half. The range of (1.47
Mev) α in boron 10 is ~ 3.3 μm.
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5.2 Problems and potential solutions
5.2.1 Problems
We encountered many problems after examining the possible final results that were difficult for
us to resolve, including the following:
1. The thickness of the used material is large in relation to the range of charged particles in
the material of interest
2. The presence of some unwanted interactions
For the second problem, it involves choosing materials that are more suitable for the detector so
that there is no unwanted result from the interaction of neutrons with these materials.
1- Neutron Filter
2- The Depleted Fuel Conversion Unit
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exploration and exploration for more uranium and increases the utilization of uranium ore in
energy production.
References
[1] P. S. Institut, "Neutron Matter Interaction," Paul Scherrer Institut, [Online]. Available:
[Link]
jwPN566jHXhEOfv2yeROdjPL5oDcSNidlJJ0hx5gXgCAw. [Accessed 2022].
[5] ResearchGate, "Variation of range as a function of kinetic energy in the zinc borophosphate
glasses," ResearchGate, jul 2021. [Online]. Available:
[Link]
the-zinc-borophosphate-glasses_fig2_352835055. [Accessed 2022].
[6] N. power, "Interactions of Neutrons with Matter," Nuclear Power, [Online]. Available:
[Link]
physics/fundamental-particles/neutron/interactions-neutrons-matter/. [Accessed 2022].
24 | P a g e
[8] americanelements, "Boron-10 Isotope," americanelements, [Online]. Available:
[Link] [Accessed 2022].
[10 H. p. Society, "Radiation shielding," Health physics Society, 2016. [Online]. Available:
] [Link] [Accessed 2022].
[15 H. X. L. H. Z. Wenrong, "Calculation of the (n,p) Reaction Cross Sections for Zinc Isotopes,"
] China Institute of Atomic Energy, Beijing.
25 | P a g e
[19 marshield, "Radiation Shielding with Lead," marshield, [Online]. Available:
] [Link] [Accessed 2022].
[20 c.-p. systems, "STAINLESS STEEL COATINGS," cor-pro systems, [Online]. Available:
] [Link] [Accessed
2022].
[21 k. metals, "WHAT IS THE STAINLESS STEEL MELTING POINT?," kloeckner metals,
] [Online]. Available: [Link]
melting-point/. [Accessed 2022].
[22 ResearchGate, "Range of alpha particles in Boron, Silicon and GaAs.," ResearchGate, 10
] 2005. [Online]. Available: [Link]
Boron-Silicon-and-GaAs_fig1_253349949. [Accessed 2022].
[24 G. E. Knoll, Radiation Detectibn and Measurement, Third ed., United States of America:
] John Wiley & Sons, Inc., 1999.
[25 J. E. Turner, Atoms, Radiation, and Radiation Protection, Third, Completely Revised and
] Enlarged Edition ed., WILEY-VCH Verlag GmbH & Co. KGaA, 2007.
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