L12 Notes-Loop
L12 Notes-Loop
Magnetic
Domain switching in Reality North-pole
On the left graph, you see snapshots of a magnetic multidomain state, that is put together
to a small video clip. By applying (external) positive and negative magnetic fields, the
magnetic domains are shifted. As this is a PDF only, you should visit the website to
see it. There is a micrometer-sized Permalloy (soft-magnetic FeNi) thin film island. On
the right, you see a (1) topography image of FIB milled Permalloy needles with two
extra magnets on the side. The rightmost image is showing the magnetic contrast of
the needle-like structures: north-poles appear dark, and south-poles appear bright. No
dynamic behavior so far, but it was made to test domain wall movement and its capturing
between the two side magnets, depending on their stray fields.
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Modeling
hierarchy
in
magnetism
If we look at dynamic behavior and its modeling, micromagnetic analysis is the most
powerful tool — at least if we consider nanomagnetic device behavior and dynamics. The
vector fields and quasi-classical description of quantum behavior by means of effective
fields (i.e. exchange interactions are described by exchange fields) is a smart way to
handle the length-scales of up to several µm.
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B B
m m
τ =mxB
vxB vxB
v v
If the magnetic induction field B is parallel to the In this case there will be a torque on the current loop
magnetic moment, then there will be no torque τ and m will make a precessional motion around B
on the current loop.
The recap should be more or less clear: angular momentum is proportionally linked to
magnetic orbital momentum.
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mr
mz
m(t)
M
Physically, dissipation is a complex multi-step process that transfers energy from the magnetic Blue arrow is the precession
degree of freedom to heat. A typical process:
1. Change in M → change in volume (Magnetostriction) → sound waves (phonons) → heat
2. Change in M → electromagnetic radiation → absorption of radiation → heat
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You can imagine, that an undamped precessional motion is not very physical. There have
to be losses and the phenomenological arguments are listed here. The damping vector
is perpendicular to the effective magnetic field Heff , summing all field contributions
like anisotropy field, exchange field, demagnetization field, Zeeman field etc. Physically
speaking, dissipation is a complex multi-step process that transfers energy from the
magnetic degree of freedom to heat.
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Typical values:
α ~ 1 for small or very rough particles (surface effects)
α ~ 0.01 – 0.1 for anisotropic metallic ferromagnets (Fe, Co, CoPt)
α ~ 0.008 for Permalloy
α ~ 0.00001 for Yttrium-Iron Garnet (YIG) M
α ~ 0.5 often used for micromagnetic simulations
Fast convergence and still some precession – it is somewhat heuristic
Energy minimum is reached when magnetization becomes parallel with the local effective field 10
Now, we are ready for the famous Landau-Lifshitz-Gilbert equation. A partial differ-
ential equation describing the time-derivative of the magnetization vector field M. We
acknowledge a precessional term (red) with magnitude γ and the damping term (blue),
with damping parameter α. The smaller α the smaller the damping, the more oscillations
are expected. For example, the YIG films in your lab course should’ve had an α in the
range of 2 × 10−4
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H eff H eff
M M
M
Top view: Top view:
The precession term makes the
magnetization going around for
forever (without changing energy)
Another summary on precession and damping terms. The LL equation is the most
important equation for micromagnetic simulations, therefore I spent many slides on it.
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Micro
Two vector fields: M (r, t ) H eff (r, t )
mag
¶M(r,t) ag é
netic
¶t
= -g M(r,t) ´ H eff (r,t) -
Ms ë
(
M(r,t) ´ M(r,t) ´ H eff (r,t) ùû )
theory
summa Landau – Lifshitz equation: how the magnetization distribution
changes under the influence of an effective field H eff (r, t )
rized
This slide highlights the clever trick of including quantum-mechanical behavior like ex-
change interaction as vector field and treating it as such in the Landau - Lifshitz equation.
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Micromagnetic modeling
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Even though, the LL equations look compact, the implementation of the LL equation
in a micromagnetic simulation tool needs quite some effort. Just to give you an idea of
what is inside of the tools available.
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Go to [Link]
→ Download the latest version under ‘Development snapshots’
For windows: just extract the zip file in a folder you like
→‘[Link]’ is the script that starts the program
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But of course, you will probably never write your own micromagnetic simulator but use
an open source or commercial tool instead. Here is a well-established software, OOMMF,
that does it for you. A bit old-fashioned but well documented.
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A second
open-source
micromag-
netic solver
mumax3
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This is a kind of newer simulator with GPU support. If you do micromagnetic simula-
tions, I can really recommend this open-source simulator — the learning curve will be
really steep.
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300nm wide
0.05
3
0
0 200 400 600 800 1000 1200 1400
Major axis [nm]
Now the question arises, how do we switch or inverse magnetization of such a single
domain magnet? Let’s look at the simulated switching field that is plotted versus the
length of the major magnet axis. For that, in step (1) a magnetic induction field B is
applied in the opposite direction to M of a single domain magnet. After that, the field
amplitude, where a reversal of magnetization occurs (2 −→ 3) is recorded. For small
major axis, we see a coherent reversal, whereas for larger magnets we see an incoherent
reversal. The higher the aspect ratio, the larger the coercivity = switching field of the
magnet. Even more, when the aspect ratio is too little, and if we are dealing with larger
magnets, incoherent reversal, and a kind of domain wall forms during reversal.
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Applied
Low aspect ratio magnet High aspect ratio magnet
field
direction Mx Mx
1.0 My 1.0 My
0.8 Mz Mz
0.8
0.6 0.6
M 0.4
0.2
0.4
0.2
B 0.0
-0.2
0.0
-0.2
-0.4 -0.4
-0.6 -0.6
-0.8 -0.8
-1.0 -1.0
-8 -6 -4 -2 0 2 4 6 8 -8 -6 -4 -2 0 2 4 6 8
Field x 10
5
5
Field x 10
1.0 Mx
My Mx
Mz 1.0 My
0.8
Mz
0.8
0.6
0.6
0.4
0.4
0.2
B 0.0
0.2
0.0
-0.2
-0.2
-0.4
-0.4
-0.6
-0.6
-0.8
-0.8
a) SEM and b) MFM images of a full
-1.0
-1.0 adder built from 53 nanomagnets.
-8 -6 -4 -2 0 2 4 6 8
Field x 10
5
-8 -6 -4 -2 0
Field
2 4 6 8
x 10
5 19
The same result as seen before, now with bar magnets and an externally applied field
(red arrow) parallel to the major axis of the magnet (top) and with some angle to the
major axis (bottom). The hysteresis loops recording Mx, My, and Mz are narrower for
tilted fields and narrower for low aspect ratio magnets. In other words, by playing with
the aspect ratio and tilted externally applied magnetic fields, we can significantly change
the switching field (coercivity) of magnets. One application was the use of magnets with
different aspect ratios in nanomagnetic logic devices from the group of the University of
Notre Dame, Indiana, USA as shown on the right.
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M M
After wall starts turning in ‘head’ After wall starts turning in ‘head’
B
B
DW moves right DW moves right
M M
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There were device proposals (and some current sensors are really using this effect), where
one plays with the movement of domain walls during reversal. Let’s look at the pin-like
shape of magnetic thin film. There is a large area acting as a nucleation region, a
magnetic strip, and a tapered hard end. This structure is injections domain walls, when
applying a magnetic field opposite to the dipole that is formed. On the left, a so-called
head-to-head domain wall is formed, on the right a tail-to-tail wall is formed, depending
on the initial magnetization and applied external field. Important here, a domain wall is
moving along the thin strip and reversing the initial dipole magnetization.
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2) Allwood et al., Science, 2002. — 3) Varga et al., IEEE Int. Conf. Nanotechnology, 2011. 21
In this science paper on the left, a famous group in GB proposed logic devices out of
such domain wall conduits (strips). By applying an in-plane rotating field, head-to-head
or tail-to-tail domain walls (DWs) were circulating, and by constrictions and correctly
chosen tapering, the type of DW was changed. The shown device is a NOT-gate, inverting
the type of wall which is the binary state (digital 0 and 1). By contrast, the devices
from Notre Dame on the right, used magnetostatic interaction between single domain
magnets to form complex gates like a 1-bit full-adder and the binary state is encoded in
the direction of the magnetization at the outputs C0 and S.
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Magnetic multi- MS
Magnetization
domain hysteresis Hc
M (r, t )
Hc
Of the many hysteresis loops I have shown you so far, this is one on the micromagnetic
scale. You can see many jumps in M when sweeping the field. But the processes are
not reversible. The two cycles are different, because, the domains form in a different
way. And the jumps you see, are the world-famous Barkhausen noise one can even see in
macroscopic hysteresis loops —- you just have to look closely (and be sensitive) enough.
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Let’s look at the previous hysteresis loop again. When talking about magnetic materials
on a macroscopic level, the magnetic permeability is a constant or proportionality factor
connecting the induced and applied induction field. In the graph on the right it is the
approximated linear fit to the hysteresis loop, but it makes only sense for small magnetic
fields until the material saturates. Hence, a differential permeability for each operating
point is often the better description. Hysteresis very generally is a phenomenon not easy
to handle, as one has to consider the history of the sample/material: complete textbooks
are written on hysteresis and how to treat it.
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æ -DE ö
E fswitching = f0 exp ç
è kT ÷ø
g Hc
kT f0 » » 0.1 GHz - 10 GHz
DE 2p
1
Tmean =
fswitching
u
First, let’s look at the limit, where ferromagnetic behavior becomes random due to el-
evated temperatures. This, we call superparamagnetic limit. Imagine, that we have a
single domain state with two possible states. It turns out, that the switching probability
follows the Arrhenius law and in order to have a stable state for more than 10 years
a barrier height of 60 kT separating the states is needed. A finding coming from HDD
research. You do not want to lose your bits earlier.
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tflip = 1 / f0
t = 1 ms
Magnetization jiggles and does not reach Particle can spontaneously flip between states
steady state
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Sweep time = 10 μs
# switching events
# switching events
Sweep time = 100 ns
Bmean = 53 mT
Bmean = 61 mT
Temperature has also an influence on switching field distributions. The slower the sweep
rate of the magnetic field in a switching experiment, the smaller the distribution (right
plot). If we sweep the magnetic field fast, the width of the distribution becomes twice
as large (left graph). Temperature helps in increasing the probability of overcoming an
energy barrier.
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[Link]
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Field interaction
An example of using the generated field of a current-carrying wire is taken from our
group. An Au strip is put on a Si-chip and the current generates a close-by field that
can be calculated. High currents, do even heat up the vicinity, which was modeled in
this work. Classical physics.
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These are the basic spin filter structures, where the orientation of the magnetic layers / external
magnetic field determines the current flowing through them. They can be used as magnetic
field sensors or for many other magneto-electronic purposes.
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A bit more complicated is this structure: a spin valve. A) A pinned ferromagnet (the
upper magnet is pinned to an anti-ferromagnet and will not switch when applying a
magnetic field), a conductor followed by a ferromagnet that can be easily switched with
magnetic fields. When now applying currents, the resistance of the structure is highly
dependent on the magnetization orientation of the two ferromagnets. B) More com-
plicated is the magnetic tunnel junction, where again a pinned and free ferromagnet
are integrated, with the difference, that a dielectric tunneling barrier is added instead
of the conductor. Tunneling in turn is dependent on the magnetic polarization of the
ferromagnetic layers.
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[Link]
spin dependent scattering
mmons/9/93/Spin-valve_GMR.svg
Low resistance High resistance
The giant magnetoresistance (GMR) was discovered in 1988 and later on, the Nobel price
was awarded for those experiments. Repetitive layers of Fe and Cr showed a big change in
magnetization depending on the orientation of the magnetization. The equivalent circuit
is shown on the right. The parallel orientation of the magnetization gives an up to 80%
reduced resistance.
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[Link]
spin dependent tunneling anti-parallel mangetisation
mmons/b/bc/TunnelSchema_TMR.svg
Low resistance High resistance
STT = Spint-transfer-torque.
Conventional vs STT-RAM Current trough MTJ is able to switch free layer.
Simpler architecture
No write line, no by-pass line and no cladding
Faster operation
Source: Driskill-Smith, Non-Volatile Memories Multibit (parallel) writing compatible
Workshop, April 2010 35
The reason for a not-scalable technology is given here for the conventional MRAM. The
write current is inversely proportional to the bit volume. The smaller the bit the larger
the current needed. But a new effect did the trick. Running a current directly through
the MTJ, a so-called spin-transfer-torque is acting on the magnetic moment, and the
switching current is proportional to the volume. That means, the smaller the cell, the
smaller the write current. STT MRAM did the trick!
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Here are the hard facts about why STT-MRAM won the race. But recently, it is the
SOT MRAM (spin-orbit-torque MRAM) that is currently overtaking.
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Even though the sketches look simple, real MTJ integration is complex. First, the MTJ
cells are fabricated AFTER all the transistors are fabricated. It is processed in the back-
end-of-line (BEOL). Magnetic materials are deposited after all diffusion barriers are put
on the chip. It puts a lot of extra processing costs on the technology. More interesting
here: The sputter-deposited magnetic layer is of crystalline nature and a lot of material
science is needed to optimize the stacks.
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• Over 200% TMR using MgO as a tunneling barrier by S Yuasa and S Parkin (2004)
• Flash memory, the embedded NVM of choice up until about 40nm process nodes, has
difficulties scaling below 28nm. For this reason the foundries Globalfoundries and Samsung
have both offered embedded MRAM options in their fully-depleted silicon-on-insulator
(FDSOI) processes. Intel embeds MRAM inFinFET process (2018, eeNEWS)
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TMR with
TMR is also in your HDD MgO barrier
Brendan A Lafferty
IMST, 2008
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TMR is not only built into recently integrated MRAM, but it was also the needed sensor
for HDD heads from 2004 on. First in a conventional, later in a MgO-TMR version. By
the way, for some months we also deposit MgO material in our sputtering tool. Difficult
material, but fun to see the results.
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Brendan A Lafferty
IMST, 2008
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The TMR layer for the HDD stack. Something for magnetic experts.
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Brendan A Lafferty
TMR is also in your HDD IMST, 2008
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And here is the proof, that it is really built into the reading head of the HDD. An SEM
image showing the tiny little tunneling barrier, probably around 1 nm thick, flying with
7200 rpm over the platter and reading the pictures you stored on your HDD. Amazing,
isn’t it?
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Brendan A Lafferty
Why we do not do TMR heads @ TUM ☺ IMST, 2008
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Take it as a joke: Such tools are used to deposit MRAM stacks or TMR heads. Huge,
expensive, and complex machines.
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This is the race track memory concept, proposed by Stuart Parkin, IBM 44
The famous Racetrack of Stuart Parkin, at that time working at IBM in California.
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And here is our concept of a 3D family of non-volatile computing elements called per-
pendicular magnetic logic. If there is time in an upcoming lecture, I am happy to talk
about it.
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Questions
Q 1:
The Landau-Lifshitz-Gilbert equation is a very famous differential equation describing
dynamics in micromagnetics. Explain the basic terms in your own words.
Q 2:
Sketch the precession of the magnetic moment M around the effective magnetic field
Heff .
Q 3:
Include the damping term in the precessional motion and compare the range of typically
used damping constants α. What is the damping constant good for?
Q 4:
In magnetism, we often deal with quantum-mechanical forces. Why is it convenient to
describe the Exchange-energy term as an Exchange-field when we are solving the LL
equation?
Q 5:
What are head-to-head and tail-to-tail domain walls? Describe an easy method/geometry
to generate those domain walls.
Q 6:
There is a family of domain-wall devices to perform logic operations with moving do-
main walls. Check the web for the original paper from Allwood at al., Submicrometer
Ferromagnetic NOT Gate and Shift Register, published in Science, 2002. What could be
the drawback of such a computation scheme with domain walls?
Q 7:
What is Barkhausen noise? What is the physical origin?
Q 8:
Having gathered experience on ferromagnetic materials and hysteretic behavior, why
should one be skeptical when discussing permeability µr as a constant number?
Q 9:
What is the superparamagnetic limit, and why is it finally limiting data retention when
scaling HDDs?
Q 10:
Coercive fields of single-domain magnetic particles are connected to the time scale of the
applied switching field (length of the applied field-pulse) by an Arrhenius law. Explain
in your own words the physics behind it.
Q 11:
Compare magnetic spin-valve and magnetic tunnel junction.
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Q 12:
Why was it impossible to scale the MRAM technology, where crossed current wires were
used to switch the magnetic bit? What effect did the trick have on novel technologies?
Explain it.
Q 13:
Explain why, in MRAM technologies, the magnetic layers are deposited in the back-
end-of-line (after all the Cu-metallization is finished) and not directly after transistor
fabrication.
Q 14:
Check the web for the latest research on racetrack memory by Stuart Parkin.